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Optical Studies of Zero-Field Magnetization of CdMnTe Quantum Dots: Influence of Average Size and Composition of Quantum Dots

机译:CdmnTe量子点零场磁化的光学研究:   量子点平均尺寸和成分的影响

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摘要

We show that through the resonant optical excitation of spin-polarizedexcitons into CdMnTe magnetic quantum dots, we can induce a macroscopicmagnetization of the Mn impurities. We observe very broad (4 meV linewidth)emission lines of single dots, which are consistent with the formation ofstrongly confined exciton magnetic polarons. Therefore we attribute theoptically induced magnetization of the magnetic dots results to the formationof spin-polarized exciton magnetic polarons. We find that the photo-inducedmagnetization of magnetic polarons is weaker for larger dots which emit atlower energies within the QD distribution. We also show that the photo-inducedmagnetization is stronger for quantum dots with lower Mn concentration, whichwe ascribe to weaker Mn-Mn interaction between the nearest neighbors within thedots. Due to particular stability of the exciton magnetic polarons in QDs,where the localization of the electrons and holes is comparable to the magneticexchange interaction, this optically induced spin alignment persists totemperatures as high as 160 K.
机译:我们表明,通过自旋极化激子共振光激发成CdMnTe磁性量子点,我们可以诱导Mn杂质的宏观磁化。我们观察到非常宽的(4 meV线宽)单点发射线,这与强约束激子磁极化子的形成是一致的。因此,我们将磁点的光感应磁化归因于自旋极化激子磁极化子的形成。我们发现,对于较大的点,其在QD分布内发出的能量较低,因此磁极化子的光感应磁化强度较弱。我们还表明,对于具有较低Mn浓度的量子点,光诱导的磁化作用更强,这归因于点内最近邻居之间的Mn-Mn相互作用较弱。由于量子点中激子磁极化子的特殊稳定性,其中电子和空穴的定位与磁交换相互作用相当,因此这种光诱导的自旋对准一直持续到160 K的高温。

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